Numerical investigation to evaluate the effects of gravity and pressure on flame structure and soot formation of turbulent non-premixed methane-air flame

Subrat Garnayak ^a, Amjad Ali Pasha ^b, Radi Alsulami ^c, Medhat A. Nemitallah ^d, Abdul Gani Abdul Jameel ^e,f, Sukanta K. Dash ^g, V. Mahendra Reddy ^g,*

a. School of Energy Science & Engineering, Indian Institute of Technology Kharagpur, West Bengal, 721302, India
         b. Department of Aerospace Engineering, King Abdulaziz University, Jeddah, 21589, Saudi Arabia
         c. Department of Mechanical Engineering, King Abdulaziz University, Jeddah, 21589, Saudi Arabia
         d. IRC-Hydrogen and Energy Storage and Mechanical Engineering Department, King Fahd University of Petroleum and Minerals, Dhahran, 31261, Saudi Arabia
         e. Department of Chemical Engineering, King Fahd University of Petroleum and Minerals, Dhahran, 31261, Saudi Arabia
         f. Center for Refining & Advanced Chemicals, King Fahd University of Petroleum and Minerals, Dhahran, 31261, Saudi Arabia
         g. Department of Mechanical Engineering, Indian Institute of Technology Kharagpur, West  Bengal, 721302, India

Abstract: In this study, a turbulent non-premixed (diffusion) methane-air flame has been investigated computationally to analyze the influences of pressure and gravity on flame structure and sooting characteristics between 1 and 10 atm. The simulation has been conducted in a 2-D axisymmetric computational domain using the finite volume-based computational fluid dynamics (CFD) code. The interaction of turbulence and chemistry is modeled by considering the steady laminar flamelet model (SLFM) and the GRI Mech 3.0 chemical mechanism. The radiative heat transfer calculation is carried out by considering the discrete ordinate (DO) method and the weighted sum grey gas model (WSGGM). The semi-empirical Moss-Brookes model is considered to calculate soot. The impact of gravity on flame and sooting characteristics are evaluated by comparing the normal-gravity flames with the zero-gravity flames. The effect of soot and radiation on flame temperature is also examined. The results show a close agreement with the measurement when both soot and radiation are included in the numerical modeling. The rates of soot formation, surface growth, and oxidation increase with increased operating pressure, regardless of gravity. Zero-gravity flames have a higher soot volume fraction, a wider soot-containing zone, a higher CO mass fraction, and a lower flame temperature than normal-gravity flames while maintaining constant pressure. In normal-gravity flames, the CO mass fraction decreases with pressure, whereas it increases with pressure rise in flames of zero gravity. Flames of zero gravity appear taller and broader compared to the flames of normal-gravity for a fixed pressure. An increase in pressure significantly reduces the flame length and width in normal-gravity flames. However, the pressure elevation has little effect on the shape of a zero-gravity flame. The outcomes of the present study will assist in fully understanding the combustion and sooting characteristics of turbulent diffusion flames that will help design and develop high-efficiency, pollutant-free combustion devices and fire suppression systems for space application.

Keywords: Computational fluid dynamics (CFD); Flamelet; Gravity; Pressure; Soot

https://doi.org/10.1016/j.jppr.2022.09.004